SREL Reprint #2442

 

Apparent decline of the sediment 137CS inventory of an abandoned reactor cooling reservoir: export or uncertainty?

 

Gregory P. Lewis, Barbara E. Taylor, John E. Pinder III, Philip M. Dixon

Savannah River Ecology Laboratory, Drawer E, Aiken, SC 29802, USA

 

Received 19 April 1999; received in revised form 12 November 1999; accepted 29 November 1999

 

Abstract

In lakes and reservoirs, variability among sediment samples can mask temporal changes in radionuclide inventories.  For Pond B, an abandoned reactor cooling reservoir in South Carolina, USA, we determined if a decline in the sediment 137CS inventory beyond radioactive decay could be detected over a 10-yr interval.  Because the 95% confidence interval for the decay-corrected change in inventory (-7.7% to + 0.8% yr-1) included 0, we could not conclusively determine that a change in inventory beyond radioactive decay had occurred.  Given the sample size of 30 pairs of sediment cores, the minimum change that could be detected reliably would have been -5.8% yr-1. By contrast, we estimate that the average export of 137Cs in surface water over the 10-yr interval was <0.6% yr-1.  For lakes and reservoirs with low rates of radionuclide export, hundreds to thousands of sediment cores may be required to detect changes in radionuclide inventories beyond radioactive decay over time spans less than several decades.  © 2000 Elsevier Science Ltd.  All rights reserved.

Keywords:  Radiocesium, 137Cs; Sediments; Lakes; Reservoir; Inventories; Remobilisation

SREL Reprint #2442

Lewis, G.P., B.E. Taylor, J.E. Pinder, III, and P.M. Dixon. 2000. Apparent decline of the sediment 137 Cs inventory of an abandoned reactor cooling reservoir:  export or uncertainty? Journal of Environmental Radioactivity 49:293-306.

 

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